The twice-widowed duchess first married aged 21 in 1947 to fellow aristocrat Luis Martinez de Irujo in a wedding on a scale to rival that of Britain's Princess Elizabeth later that year.
Wearing a pearl and diamond crown, she rode to Seville Cathedral in a horse-drawn carriage with thousands of well-wishers lining the streets to cheer her. The couple had six children.
She became a fixture of the international jet-set, hosting Audrey Hepburn and Jackie Kennedy on their visits to Spain and turning her Madrid palace over to French designer Yves Saint Laurent to stage a Dior fashion show in 1959.
An aficionado of bull-fighting and flamenco, she often took place of honor at bull-fights in her beloved Seville, usually sporting a magnificent 'mantilla' - the traditional Spanish lace veil worn over a high comb.
The duchess, who favored an eccentric clothing style, sporting beaded anklets and fishnet tights well into her eighties, married former Catholic priest Jesus Aguirre Ortiz de Zarate six years after the death of her first husband.
Her second husband died in 2001. Her courtship with dashing civil servant Alfonso Diez gripped the nation, aroused disapproval from Queen Sofia and was openly opposed by her six children.
Before tying the knot with 61-year-old Diez in 2011, the duchess divided her fortune between her offspring to silence their protests.
Although ill health kept her out of the public eye in later months, her most memorable recent image was when she flung off her shoes to perform an impromptu flamenco dance before a forest of cameras and well-wishers at her third wedding.
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